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[摘要]:The angular dependencies of the local field enhancement and the Raman emission enhancement are investigated, numerically and experimentally, for a plasmonic crystal double resonance SERS substrate consisting of a periodic array of gold disks above a gold film. We find that the local field enhancement is very sensitive to the incident angle. The Raman emission enhancement has a strong angular dependence on the detection direction, with the substrate "beaming" the Raman emission so that different Raman lines have different far-field patterns. We demonstrate that a stronger SERS signal results when the plasmonic substrate is illuminated with a collimated, rather than focused, laser beam. (C) 2011 Optical Society of America |
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