Intramolecular Chemoselective Acylation of a Suitably Substituted Isoindole: Synthesis of (+/-)-Chilenine and (+/-)-Deoxychilenine

[摘要]：Starting from 3,4-dimethoxyhomophthalic anhydride and 6-bromohomopiperonylamine, concise and efficient syntheses of Chilean berberis products chilenine and deoxychilenine have been demonstrated via partially divergent routes by taking advantage of facile air-oxidation of homophthalimide along with intramolecular chemoselective acylation as the key steps.

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