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Palladium Induced Macrocyclic Preorganization for Stabilization of a Tetrathiafulvalene Mixed-Valence Dimer

  作者 BEJGER CHRISTOPHER; DAVIS CHRISTINA M; PARK JUNG SU; LYNCH VINCENT M; LOVE JASON B; SESSLER JONATHAN L  
  选自 期刊  Organic Letters;  卷期  2011年13-18;  页码  4902-4905  
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[摘要]Ditopic metalation of a flexible "Pacman"-like tetrathiafulvalene (TTF) modified Schiff-base-calixpyrrole results in the stabilization upon oxidation of an otherwise difficult-to-access mixed-valence TTF radical dimer. EPR and optical spectroscopies were used to characterize the mixed-valence species.

 
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