Polycyclic Imide Derivatives: Synthesis and Effective Tuning of Lowest Unoccupied Molecular Orbital Levels through Molecular Engineering

[摘要]：A series of fluoranthene-fused imide derivatives were facilely developed through a Diels-Alder reaction followed by decarbonylation. The investigation of their photophysical and electrochemical properties demonstrated that their LUMO levels were effectively tuned from -3.2 to -3.8 eV through the introduction of a fused imide unit, which provides a platform to design new air-stable and solution-processable n-type materials.

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