Organocatalytic approach to benzofused nitrogen-containing heterocycles: enantioselective total synthesis of (+)-Angustureine.

[摘要]：The organocatalytic intramol. aza-Michael reaction (IMAMR) was employed as an enantioselective tool to generate enantiomerically enriched isoindolines, indolines, tetrahydroquinolines, and tetrahydroisoquinolines from o-substituted alkylidenes, anilines and benzylamines. The methodol. was applied to the synthesis of the natural product (+)-angustureine (I).

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