Organocatalyzed enantioselective synthesis of nitroalkanes bearing all-carbon quaternary stereogenic centers through conjugate addition of acetone cyanohydrin.

[摘要]：The first organocatalyzed phase-transfer enantioselective conjugate addn. of cyanide ion derived from acetone cyanohydrin to b,b'-disubstituted nitro olefins is reported. The reaction leads to the efficient formation of nitro alkanes bearing an all-C quaternary stereogenic center in ?2% ee.

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