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Surface-Plasmon-Induced Modification on the Spontaneous Emission Spectrum via Subwavelength-Confined Anisotropic Purcell Factor

  作者 Gu, Y; Wang, LJ; Ren, P; Zhang, JX; Zhang, TC; Martin, OJF; Gong, QH  
  选自 期刊  Nano Letters;  卷期  2012年12-5;  页码  2488-2493  
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[摘要]The mechanism of using the anisotropic Purcell factor to control the spontaneous emission linewidths in a four-level atom is theoretically demonstrated; if the polarization angle bisector of the two dipole moments lies along the axis of large/small Purcell factor, destructive/constructive interference narrows/widens the fluorescence center spectral lines. Large anisotropy of the Purcell factor, confined in the subwavelength optical mode volume, leads to rapid spectral line narrowing of atom approaching a metallic nanowire, nanoscale line width pulsing following periodically varying decay rates near a periodic metallic nanostructure, and dramatic modification on the spontaneous emission spectrum near a custom-designed resonant plasmon nanostructure. The combined system opens a good perspective for applications in ultracompact active quantum devices.

 
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