Direct Substitution of Hydroxy Group of pi-Activated Alcohols with Electron-Deficient Amines Using Re2O7 Catalyst

[摘要]：The first example of simple Re2O7-catalyzed direct dehydrative coupling between allylic alcohols with electron-deficient amines has been achieved under mild and open flask conditions. The protocol has also been successfully applied to benzylic and propargylic alcohols. The mechanistic proof for the S(N)1-type process has also been provided.

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