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Dramatic thermal conductivity reduction by nanostructures for large increase in thermoelectric figure-of-merit of FeSb2 - art. no. 163101

  作者 Zhao, HZ; Pokheral, M; Zhu, GH; Chen, S; Lukas, K; Jie, Q; Opeil, C; Chen, G; Ren, ZF  
  选自 期刊  Applied Physics Letters;  卷期  2011年99-16;  页码  63101-63101  
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[摘要]In this report, thermal conductivity reduction by more than three orders of magnitude over its single crystal counterpart for the strongly correlated system FeSb2 through a nanostructure approach was presented, leading to a significant increase of thermoelectric figure-of-merit (ZT). For the samples processed with the optimal parameters, the thermal conductivity reached 0.34Wm(-1) K-1 at 50 K, leading to a ZT peak of about 0.013, compared to 0.005 for single crystal FeSb2, an increase of about 160%. This work suggests that nanostructure method is effective and can be possibly extended to other strongly correlated low temperature thermoelectric materials, paving the way for future cryogenic temperature cooling applications. (C) 2011 American Institute of Physics. [doi:10.1063/1.3651757]

 
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