Surface adsorption and disordering in LiFePO4 based battery cathodes

[摘要]：A recent study [Kang and Ceder, Nature (London) 458, 190 (2009)] suggested that a Li4P2O7-like "fast ion-conducting surface phase" could form on the surfaces of LiFePO4 particles, enabling ultrafast discharging of Li-ion batteries. We demonstrate that the

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