Biradical Character of Linear pi-Conjugated Oligomer Dications Composed of Thiophene, Pyrrole, and Methylthio End-Capping Units

[摘要]：Combined DFT calculations and UV-vis-NIR, ESR, and SQUID measurements revealed that the ground-state electronic structure of a linear pi-conjugated oligomer dication composed of two pyrrole and six or seven thiophene rings and methylthio end-capping units is dominated by a singlet biradical character.

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